@article{ART002845080},
author={Kou Xiaoli and Xin Xin and Zhang Yan and Meng Long-Yue},
title={Facile synthesis of nitrogen-doped carbon dots (N-CDs) and N-CDs/NiO composite as an efficient electrocatalyst for oxygen evolution reaction},
journal={Carbon Letters},
issn={1976-4251},
year={2021},
volume={31},
number={4},
pages={695-706},
doi={10.1007/s42823-021-00255-0}
TY - JOUR
AU - Kou Xiaoli
AU - Xin Xin
AU - Zhang Yan
AU - Meng Long-Yue
TI - Facile synthesis of nitrogen-doped carbon dots (N-CDs) and N-CDs/NiO composite as an efficient electrocatalyst for oxygen evolution reaction
JO - Carbon Letters
PY - 2021
VL - 31
IS - 4
PB - Korean Carbon Society
SP - 695
EP - 706
SN - 1976-4251
AB - Nitrogen-doped carbon dots (N-CDs), derived from the biomass (anthocyanin), are the novel additive to the nanocarbon materials, which is expected to bring a wide spectrum of novel applications. Moreover, metallic oxides are emerging for their unique potential for electrocatalysis. Herein, we report the synthesis of N-CDs for the selective detection of Fe3+ with a limit of detection of 2.57 μM in the range of 5–60 μM using ethylenediamine and H2O2 by a hydrothermal method. The obtained N-CDs displayed a spherical morphology with a particle size range of 2–7 nm and emitted blue luminescence at 394 nm under excitation at 319 nm. Meanwhile, we have demonstrated the fabrication of cost-efcient electrocatalysts for oxygen evolution reaction (OER) in an alkaline medium, employing N-CDs. Owing to the successful incorporation of N-CDs into NiO nanospheres, the resulting N-CDs/NiO with large surface areas, fast charge transfer, and increased conductivity vastly improved the catalytic activity. Remarkably, the optimal of N-CDs/NiO composite requires the overpotential of only 380 mV at a current density of 10 mA cm−2 and a relatively low Tafel slope of 57.96 mV dec−1 compared with pure NiO. These results open up a facile route for the application of N-CDs and ofer prospects for CD-metal hybrids as high OER catalysts in electrochemical energy devices.
KW - Nitrogen-doped carbon dots · Anthocyanin · NiO · Oxygen evolution reaction · Electrocatalysts
DO - 10.1007/s42823-021-00255-0
ER -
Kou Xiaoli, Xin Xin, Zhang Yan and Meng Long-Yue. (2021). Facile synthesis of nitrogen-doped carbon dots (N-CDs) and N-CDs/NiO composite as an efficient electrocatalyst for oxygen evolution reaction. Carbon Letters, 31(4), 695-706.
Kou Xiaoli, Xin Xin, Zhang Yan and Meng Long-Yue. 2021, "Facile synthesis of nitrogen-doped carbon dots (N-CDs) and N-CDs/NiO composite as an efficient electrocatalyst for oxygen evolution reaction", Carbon Letters, vol.31, no.4 pp.695-706. Available from: doi:10.1007/s42823-021-00255-0
Kou Xiaoli, Xin Xin, Zhang Yan, Meng Long-Yue "Facile synthesis of nitrogen-doped carbon dots (N-CDs) and N-CDs/NiO composite as an efficient electrocatalyst for oxygen evolution reaction" Carbon Letters 31.4 pp.695-706 (2021) : 695.
Kou Xiaoli, Xin Xin, Zhang Yan, Meng Long-Yue. Facile synthesis of nitrogen-doped carbon dots (N-CDs) and N-CDs/NiO composite as an efficient electrocatalyst for oxygen evolution reaction. 2021; 31(4), 695-706. Available from: doi:10.1007/s42823-021-00255-0
Kou Xiaoli, Xin Xin, Zhang Yan and Meng Long-Yue. "Facile synthesis of nitrogen-doped carbon dots (N-CDs) and N-CDs/NiO composite as an efficient electrocatalyst for oxygen evolution reaction" Carbon Letters 31, no.4 (2021) : 695-706.doi: 10.1007/s42823-021-00255-0
Kou Xiaoli; Xin Xin; Zhang Yan; Meng Long-Yue. Facile synthesis of nitrogen-doped carbon dots (N-CDs) and N-CDs/NiO composite as an efficient electrocatalyst for oxygen evolution reaction. Carbon Letters, 31(4), 695-706. doi: 10.1007/s42823-021-00255-0
Kou Xiaoli; Xin Xin; Zhang Yan; Meng Long-Yue. Facile synthesis of nitrogen-doped carbon dots (N-CDs) and N-CDs/NiO composite as an efficient electrocatalyst for oxygen evolution reaction. Carbon Letters. 2021; 31(4) 695-706. doi: 10.1007/s42823-021-00255-0
Kou Xiaoli, Xin Xin, Zhang Yan, Meng Long-Yue. Facile synthesis of nitrogen-doped carbon dots (N-CDs) and N-CDs/NiO composite as an efficient electrocatalyst for oxygen evolution reaction. 2021; 31(4), 695-706. Available from: doi:10.1007/s42823-021-00255-0
Kou Xiaoli, Xin Xin, Zhang Yan and Meng Long-Yue. "Facile synthesis of nitrogen-doped carbon dots (N-CDs) and N-CDs/NiO composite as an efficient electrocatalyst for oxygen evolution reaction" Carbon Letters 31, no.4 (2021) : 695-706.doi: 10.1007/s42823-021-00255-0