Carbon Letters 2023 KCI Impact Factor : 1.35 KCI-WoS Impact Factor : 6.04
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pISSN : 1976-4251 / eISSN : 2233-4998
- https://journal.kci.go.kr/carbon
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Gamma-ray irradiated graphene nanosheets/polydopamine hybrids as a superior anode material for lithium-ion batteries
- Carbon Letters
- Abbr : Carbon Lett.
- 2022, 32(1), pp.305-312
- DOI : 10.1007/s42823-021-00308-4
- Publisher : Korean Carbon Society
- Research Area : Natural Science > Natural Science General > Other Natural Sciences General
- Received : July 15, 2021
- Accepted : November 15, 2021
- Published : January 1, 2022
Jo Kyoung-Il 1, Kim Hyeri 2, Jeong Hee-Sung 2, KEE JIN HO 3, Oh Seung-Hwan 2, Song Seok Hyun 4, Kim Hyungsub 5, Koo Jaseung 2
1한국원자력연구원
2충남대학교 유기재료공학과
3충남대학교
4고려대학교 화학생물공학과
5한국원자력연구원 중성자과학부
Accredited
ABSTRACT
Despite having a low electrical conductivity, graphene oxide (GO) is used as an anode material in lithium-ion batteries (LIBs) owing its good processability in large quantities. GO is reduced by chemical or thermal treatments to enhance its electrical conductivity. In this study, high-performance GO anodes with polydopamine (PDA) and polyethylenimine (PEI) as binders were fabricated. Gamma (γ)-ray irradiation was applied to the GO–PDA–PEI hybrid sheets to covalently cross-link the GO sheets and binders with an amide bond. The covalent crosslinking was confirmed by Fourier-transform infrared spectroscopy analysis. Further, X-ray photoelectron spectroscopy results showed that γ-ray irradiation produced a reduced GO sheet, which resulted in an increase in the electrical conductivity by 30%. By characterizing the electrochemical properties, we found that the γ-ray irradiation facilitates the stability and increases the charge/discharge capacity by crosslinking GO and PDA–PEI binders and reducing the GO sheets.
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This paper was written with support from the National Research Foundation of Korea.