@article{ART002959003},
author={Jiang Ye and Wan Sijie and Zhao Weiwei and Yu Wenjie and Wang Shuaipeng and Yu Zeqi and Yang Qiu and Zhou Weihua and Liu Xiaoqing},
title={Reusable, magnetic laser-induced graphene for efficient removal of organic pollutants from water},
journal={Carbon Letters},
issn={1976-4251},
year={2022},
volume={32},
number={4},
pages={1047-1064},
doi={10.1007/s42823-022-00336-8}
TY - JOUR
AU - Jiang Ye
AU - Wan Sijie
AU - Zhao Weiwei
AU - Yu Wenjie
AU - Wang Shuaipeng
AU - Yu Zeqi
AU - Yang Qiu
AU - Zhou Weihua
AU - Liu Xiaoqing
TI - Reusable, magnetic laser-induced graphene for efficient removal of organic pollutants from water
JO - Carbon Letters
PY - 2022
VL - 32
IS - 4
PB - Korean Carbon Society
SP - 1047
EP - 1064
SN - 1976-4251
AB - The hybridization of graphene with magnetic nanoparticles has endowed graphene with increasing interest as the adsorbent for wastewater treatment. However, its fabrication often involves a multi-stepped chemical synthesis process. In this work, we demonstrate a facile, one-step, and solvent-free approach to fabricate Fe3O4 nanoparticle-anchored Laser-Induced Graphene (Fe3O4@LIG) as an efficient adsorbent by direct laser irradiation on a ferric acetylacetonate containing polybenzoxazine film. Raman and X-ray diffraction analysis confirm the graphene component in the adsorbent, and the morphology characterizations show that Fe3O4 nanoparticles are distributed uniformly on LIG with hierarchical meso- and macro-porous structures. Adsorption experiments indicate that Fe3O4@LIG can adsorb methylene blue (MB) from aqueous solutions in a fast and effective manner, with a maximum adsorption capacity up to 350.9 mg/g. The adsorption kinetics and isotherms are also investigated, which are well-described by the pseudo-second-order model and Langmuir model, respectively. Additionally, Fe3O4@LIG is also demonstrated with the efficient removal of a variety of organic solvents from water. The favorable adsorption behavior of Fe3O4@LIG is attributed to its unique porous structure and the molecular interactions with adsorbates. On the other hand, Fe3O4@LIG has high magnetic property, and therefore, it could be easily recovered from water and well regenerated for repeated use. With the efficient adsorption of organic pollutants, magnetic separability, and good recyclability, it is believed that the easy-fabricated Fe3O4@LIG has great potential applications in wastewater treatment.
KW - Laser-induced graphene Magnetic Adsorption Methylene blue Organic solvents
DO - 10.1007/s42823-022-00336-8
ER -
Jiang Ye, Wan Sijie, Zhao Weiwei, Yu Wenjie, Wang Shuaipeng, Yu Zeqi, Yang Qiu, Zhou Weihua and Liu Xiaoqing. (2022). Reusable, magnetic laser-induced graphene for efficient removal of organic pollutants from water. Carbon Letters, 32(4), 1047-1064.
Jiang Ye, Wan Sijie, Zhao Weiwei, Yu Wenjie, Wang Shuaipeng, Yu Zeqi, Yang Qiu, Zhou Weihua and Liu Xiaoqing. 2022, "Reusable, magnetic laser-induced graphene for efficient removal of organic pollutants from water", Carbon Letters, vol.32, no.4 pp.1047-1064. Available from: doi:10.1007/s42823-022-00336-8
Jiang Ye, Wan Sijie, Zhao Weiwei, Yu Wenjie, Wang Shuaipeng, Yu Zeqi, Yang Qiu, Zhou Weihua, Liu Xiaoqing "Reusable, magnetic laser-induced graphene for efficient removal of organic pollutants from water" Carbon Letters 32.4 pp.1047-1064 (2022) : 1047.
Jiang Ye, Wan Sijie, Zhao Weiwei, Yu Wenjie, Wang Shuaipeng, Yu Zeqi, Yang Qiu, Zhou Weihua, Liu Xiaoqing. Reusable, magnetic laser-induced graphene for efficient removal of organic pollutants from water. 2022; 32(4), 1047-1064. Available from: doi:10.1007/s42823-022-00336-8
Jiang Ye, Wan Sijie, Zhao Weiwei, Yu Wenjie, Wang Shuaipeng, Yu Zeqi, Yang Qiu, Zhou Weihua and Liu Xiaoqing. "Reusable, magnetic laser-induced graphene for efficient removal of organic pollutants from water" Carbon Letters 32, no.4 (2022) : 1047-1064.doi: 10.1007/s42823-022-00336-8
Jiang Ye; Wan Sijie; Zhao Weiwei; Yu Wenjie; Wang Shuaipeng; Yu Zeqi; Yang Qiu; Zhou Weihua; Liu Xiaoqing. Reusable, magnetic laser-induced graphene for efficient removal of organic pollutants from water. Carbon Letters, 32(4), 1047-1064. doi: 10.1007/s42823-022-00336-8
Jiang Ye; Wan Sijie; Zhao Weiwei; Yu Wenjie; Wang Shuaipeng; Yu Zeqi; Yang Qiu; Zhou Weihua; Liu Xiaoqing. Reusable, magnetic laser-induced graphene for efficient removal of organic pollutants from water. Carbon Letters. 2022; 32(4) 1047-1064. doi: 10.1007/s42823-022-00336-8
Jiang Ye, Wan Sijie, Zhao Weiwei, Yu Wenjie, Wang Shuaipeng, Yu Zeqi, Yang Qiu, Zhou Weihua, Liu Xiaoqing. Reusable, magnetic laser-induced graphene for efficient removal of organic pollutants from water. 2022; 32(4), 1047-1064. Available from: doi:10.1007/s42823-022-00336-8
Jiang Ye, Wan Sijie, Zhao Weiwei, Yu Wenjie, Wang Shuaipeng, Yu Zeqi, Yang Qiu, Zhou Weihua and Liu Xiaoqing. "Reusable, magnetic laser-induced graphene for efficient removal of organic pollutants from water" Carbon Letters 32, no.4 (2022) : 1047-1064.doi: 10.1007/s42823-022-00336-8