Core–shell ZIF-67(Co) wrapped CuO as high efficient peroxymonosulfate catalyst for the degradation of methylene blue

Zhu Wenjun; Zuo Xiaohua; Deng Xiangyi; Zhang Xinhao; Yao Chuang; Wang Xiaobo

doi:10.1007/s42823-022-00446-3

Core–shell ZIF-67(Co) wrapped CuO as high efficient peroxymonosulfate catalyst for the degradation of methylene blue

Carbon Letters
Abbr : Carbon Lett.
2023, 33(2), pp.573-585
DOI : 10.1007/s42823-022-00446-3
Publisher : Korean Carbon Society
Research Area : Natural Science > Natural Science General > Other Natural Sciences General
Received : August 17, 2022
Accepted : December 2, 2022
Published : March 1, 2023

Zhu Wenjun ¹, Zuo Xiaohua ², Deng Xiangyi ², Zhang Xinhao ², Yao Chuang ³, Wang Xiaobo ⁴

¹Hubei Key Laboratory of Coal Conversion and New Carbon Material, School of Chemistry and Chemical Engineering, Wuhan University of Science and Technology, Wuhan
²College of Chemistry and Chemical Engineering, Hubei Key Laboratory of Mine Environmental Pollution Control and Remediation, Hubei Polytechnic University
³Guangdong Wastewater Treatment Engineering Technology Center of Standard and Efficiency Increasing and Resource Recycling, Guagdong Research Institute of Engineering Technology Co.
⁴College of Chemistry and Chemical Engineering, Hubei Key Laboratory of Mine Environmental Pollution Control and Remediation, Hubei Polytechnic University, Huangshi

Accredited

ABSTRACT

Core–shell ZIFs wrapped CuO hybrid materials (CuO@ZIF-67(Co)) were designed, synthesized, characterized, and employed as peroxymonosulfate (PMS) activators to degrade methylene blue (MB). It demonstrated outstanding catalytic activity on account of the unique structure and the synergistic effect between CuO cores and ZIF-67(Co) shells, resulting in complete degradation of MB (10 mg/L) in 1 min. Reactive oxygen species (ROSs) research showed that both SO4− and OH were responsible for the removal of MB. The synergistic activation mechanisms in the CuO@ZIF-67(Co)/PMS system were investigated, which mainly involved the effective electron transfer of CuO and ZIF-67(Co) for accelerating the cycle of CuII/CuI and CoIII/CoII. This study broadens the application of MOF-derived materials for wastewater treatment.

KEYWORDS

MOFs Degradation Peroxymonosulfate Methylene blue

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Carbon Letters 2023 KCI Impact Factor : 1.35 KCI-WoS Impact Factor : 6.04

Core–shell ZIF-67(Co) wrapped CuO as high efficient peroxymonosulfate catalyst for the degradation of methylene blue

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This is the result of checking the information with the same ISSN, publication year, volume, and start page between the WoS and the KCI journals. (as of 2024-07-26)

Total Citation Counts(KCI+WOS) (1) This is the number of times that the duplicate count has been removed by comparing the citation list of WoS and KCI.

Scopus Citation Counts (1) This is the result of checking the information with the same ISSN, publication year, volume, and start page between articles in KCI and the SCOPUS journals. (as of 2024-10-01)

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Carbon Letters 2023 KCI Impact Factor : 1.35 KCI-WoS Impact Factor : 6.04

Core–shell ZIF-67(Co) wrapped CuO as high efficient peroxymonosulfate catalyst for the degradation of methylene blue

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Total Citation Counts(KCI+WOS) (1) This is the number of times that the duplicate count has been removed by comparing the citation list of WoS and KCI.

Scopus Citation Counts (1) This is the result of checking the information with the same ISSN, publication year, volume, and start page between articles in KCI and the SCOPUS journals. (as of 2024-10-01)

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