@article{ART003185720},
author={Lee, Jaegeun},
title={Data analytics approach to evaluating the impact of acetylene and ethylene precursors on the crystallinity of carbon nanotubes synthesized in a fluidized bed reactor},
journal={Carbon Letters},
issn={1976-4251},
year={2025},
volume={35},
number={1},
pages={199-209},
doi={10.1007/s42823-024-00782-6}
TY - JOUR
AU - Lee, Jaegeun
TI - Data analytics approach to evaluating the impact of acetylene and ethylene precursors on the crystallinity of carbon nanotubes synthesized in a fluidized bed reactor
JO - Carbon Letters
PY - 2025
VL - 35
IS - 1
PB - Korean Carbon Society
SP - 199
EP - 209
SN - 1976-4251
AB - The mass production of highly crystalline carbon nanotubes (CNTs) is highly demanded, yet achieving it remains challenging due to incomplete understanding of how synthetic parameters, except temperature, affect the crystallinity of CNTs. Notably, the choice of carbon precursor significantly influences CNT synthesis, but its impact on crystallinity remains unclear. Here, we employed a data analytics approach to examine the effect of carbon precursors on CNT crystallinity during their synthesis in a fluidized bed reactor. We compared ethylene, acetylene, and a mixture of these. Using Bayesian optimization (BO), we optimized synthesis conditions to maximize IG/ID of CNTs for each precursor. Key parameters considered were reaction temperature, precursor concentration, and hydrogen concentration. We conducted three separate BO processes to evaluate the effectiveness of each carbon precursor on CNT crystallinity. The results indicated no significant difference in IG/ID of CNTs among the carbon precursors. In addition, multiple linear regression analysis did not support a synergetic effect between acetylene and ethylene. Interestingly, contour plots demonstrated consistent relationships between synthesis parameters and IG/ID across different carbon precursors. This data analytics approach allowed us to successfully assess the impact of carbon precursors on the CNT crystallinity and analyze the relationship between synthesis parameters and CNT crystallinity.
KW - Carbon nanotubes Catalyst Bayesian optimization Crystallinity Carbon precursor Fluidized bed reactor
DO - 10.1007/s42823-024-00782-6
ER -
Lee, Jaegeun. (2025). Data analytics approach to evaluating the impact of acetylene and ethylene precursors on the crystallinity of carbon nanotubes synthesized in a fluidized bed reactor. Carbon Letters, 35(1), 199-209.
Lee, Jaegeun. 2025, "Data analytics approach to evaluating the impact of acetylene and ethylene precursors on the crystallinity of carbon nanotubes synthesized in a fluidized bed reactor", Carbon Letters, vol.35, no.1 pp.199-209. Available from: doi:10.1007/s42823-024-00782-6
Lee, Jaegeun "Data analytics approach to evaluating the impact of acetylene and ethylene precursors on the crystallinity of carbon nanotubes synthesized in a fluidized bed reactor" Carbon Letters 35.1 pp.199-209 (2025) : 199.
Lee, Jaegeun. Data analytics approach to evaluating the impact of acetylene and ethylene precursors on the crystallinity of carbon nanotubes synthesized in a fluidized bed reactor. 2025; 35(1), 199-209. Available from: doi:10.1007/s42823-024-00782-6
Lee, Jaegeun. "Data analytics approach to evaluating the impact of acetylene and ethylene precursors on the crystallinity of carbon nanotubes synthesized in a fluidized bed reactor" Carbon Letters 35, no.1 (2025) : 199-209.doi: 10.1007/s42823-024-00782-6
Lee, Jaegeun. Data analytics approach to evaluating the impact of acetylene and ethylene precursors on the crystallinity of carbon nanotubes synthesized in a fluidized bed reactor. Carbon Letters, 35(1), 199-209. doi: 10.1007/s42823-024-00782-6
Lee, Jaegeun. Data analytics approach to evaluating the impact of acetylene and ethylene precursors on the crystallinity of carbon nanotubes synthesized in a fluidized bed reactor. Carbon Letters. 2025; 35(1) 199-209. doi: 10.1007/s42823-024-00782-6
Lee, Jaegeun. Data analytics approach to evaluating the impact of acetylene and ethylene precursors on the crystallinity of carbon nanotubes synthesized in a fluidized bed reactor. 2025; 35(1), 199-209. Available from: doi:10.1007/s42823-024-00782-6
Lee, Jaegeun. "Data analytics approach to evaluating the impact of acetylene and ethylene precursors on the crystallinity of carbon nanotubes synthesized in a fluidized bed reactor" Carbon Letters 35, no.1 (2025) : 199-209.doi: 10.1007/s42823-024-00782-6
