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@article{ART003208662},
author={Ehsan Vafa and Mohammad Barghamadi and Somayeh Parham and Katayoon Rezaeeparto and Mohammad Bagher Zarei and Mohammad Javad Azizli and Mohammad Ali Amani and Hesam Kamyab and Shreeshivadasan Chelliapan},
title={Graphene oxide-enhanced multiscale modeling of PGDLLA/P(lLA-co-ɛ-CL)/PCL interfacial debonding: investigating rheological and mechanical properties, compatibility, and morphology},
journal={Carbon Letters},
issn={1976-4251},
year={2025},
volume={35},
number={2},
pages={553-573},
doi={10.1007/s42823-024-00793-3}

TY - JOUR
AU - Ehsan Vafa
AU - Mohammad Barghamadi
AU - Somayeh Parham
AU - Katayoon Rezaeeparto
AU - Mohammad Bagher Zarei
AU - Mohammad Javad Azizli
AU - Mohammad Ali Amani
AU - Hesam Kamyab
AU - Shreeshivadasan Chelliapan
TI - Graphene oxide-enhanced multiscale modeling of PGDLLA/P(lLA-co-ɛ-CL)/PCL interfacial debonding: investigating rheological and mechanical properties, compatibility, and morphology
JO - Carbon Letters
PY - 2025
VL - 35
IS - 2
PB - Korean Carbon Society
SP - 553
EP - 573
SN - 1976-4251
AB - In this paper, poly(glycolic acid–co-DL–lactic acid) (PGDLLA)/poly(ɛ-caprolactone) (PCL) incompatible nanocomposites were combined with multiscale modeling (MSM) in a ratio of 80/20. Since the behavior and mechanical properties of blends depend significantly on the interphase region, the compatibilizer poly(l,l-lactic acid–co-ɛ-caprolactone) (P(lLA-co-ɛ-CL)) was used to improve compatibility and graphene oxide (GO) was used to increase the interphase strength of PGDLLA matrix/PCL. This work was done by mixing solvent to achieve the optimum disperse of GO in the matrix. The investigation of interfacial phenomenon by the theoretical interfacial models is important. Under the assumption of constant modulus and elastic deformation in the zero interface region, the predictions in this region are more unreliable when the calculations of experimental mechanical properties are analyzed in detail. In this study, PGDLLA/P(lLA-co-ɛ-CL)/PCL compounds were compared with the MSM approach to predict the plastic deformation in the stress–strain behavior. In contrast to the hypothesis that a simple look at the interphase area in nanocomposites, a finite element code is proposed to evaluate the efficiency of the interphase area. Both experimental results and FEM analysis showed that Young’s modulus increases by incorporating GO into GO/PGDLLA/P(lLA-co-ɛ-CL)/PCL nanocomposites; the amount of increase for incorporating 1 phr GO is about 61%.
KW - Multiscale modeling;Interface region;Graphene oxide;PGDLLA/P(lLA-co-ɛ-CL)/PCL
DO - 10.1007/s42823-024-00793-3
ER -

Ehsan Vafa, Mohammad Barghamadi, Somayeh Parham, Katayoon Rezaeeparto, Mohammad Bagher Zarei, Mohammad Javad Azizli, Mohammad Ali Amani, Hesam Kamyab and Shreeshivadasan Chelliapan. (2025). Graphene oxide-enhanced multiscale modeling of PGDLLA/P(lLA-co-ɛ-CL)/PCL interfacial debonding: investigating rheological and mechanical properties, compatibility, and morphology. Carbon Letters, 35(2), 553-573.

Ehsan Vafa, Mohammad Barghamadi, Somayeh Parham, Katayoon Rezaeeparto, Mohammad Bagher Zarei, Mohammad Javad Azizli, Mohammad Ali Amani, Hesam Kamyab and Shreeshivadasan Chelliapan. 2025, "Graphene oxide-enhanced multiscale modeling of PGDLLA/P(lLA-co-ɛ-CL)/PCL interfacial debonding: investigating rheological and mechanical properties, compatibility, and morphology", Carbon Letters, vol.35, no.2 pp.553-573. Available from: doi:10.1007/s42823-024-00793-3

Ehsan Vafa, Mohammad Barghamadi, Somayeh Parham, Katayoon Rezaeeparto, Mohammad Bagher Zarei, Mohammad Javad Azizli, Mohammad Ali Amani, Hesam Kamyab, Shreeshivadasan Chelliapan "Graphene oxide-enhanced multiscale modeling of PGDLLA/P(lLA-co-ɛ-CL)/PCL interfacial debonding: investigating rheological and mechanical properties, compatibility, and morphology" Carbon Letters 35.2 pp.553-573 (2025) : 553.

Ehsan Vafa, Mohammad Barghamadi, Somayeh Parham, Katayoon Rezaeeparto, Mohammad Bagher Zarei, Mohammad Javad Azizli, Mohammad Ali Amani, Hesam Kamyab, Shreeshivadasan Chelliapan. Graphene oxide-enhanced multiscale modeling of PGDLLA/P(lLA-co-ɛ-CL)/PCL interfacial debonding: investigating rheological and mechanical properties, compatibility, and morphology. 2025; 35(2), 553-573. Available from: doi:10.1007/s42823-024-00793-3

Ehsan Vafa, Mohammad Barghamadi, Somayeh Parham, Katayoon Rezaeeparto, Mohammad Bagher Zarei, Mohammad Javad Azizli, Mohammad Ali Amani, Hesam Kamyab and Shreeshivadasan Chelliapan. "Graphene oxide-enhanced multiscale modeling of PGDLLA/P(lLA-co-ɛ-CL)/PCL interfacial debonding: investigating rheological and mechanical properties, compatibility, and morphology" Carbon Letters 35, no.2 (2025) : 553-573.doi: 10.1007/s42823-024-00793-3

Ehsan Vafa; Mohammad Barghamadi; Somayeh Parham; Katayoon Rezaeeparto; Mohammad Bagher Zarei; Mohammad Javad Azizli; Mohammad Ali Amani; Hesam Kamyab; Shreeshivadasan Chelliapan. Graphene oxide-enhanced multiscale modeling of PGDLLA/P(lLA-co-ɛ-CL)/PCL interfacial debonding: investigating rheological and mechanical properties, compatibility, and morphology. Carbon Letters, 35(2), 553-573. doi: 10.1007/s42823-024-00793-3

Ehsan Vafa; Mohammad Barghamadi; Somayeh Parham; Katayoon Rezaeeparto; Mohammad Bagher Zarei; Mohammad Javad Azizli; Mohammad Ali Amani; Hesam Kamyab; Shreeshivadasan Chelliapan. Graphene oxide-enhanced multiscale modeling of PGDLLA/P(lLA-co-ɛ-CL)/PCL interfacial debonding: investigating rheological and mechanical properties, compatibility, and morphology. Carbon Letters. 2025; 35(2) 553-573. doi: 10.1007/s42823-024-00793-3

Ehsan Vafa, Mohammad Barghamadi, Somayeh Parham, Katayoon Rezaeeparto, Mohammad Bagher Zarei, Mohammad Javad Azizli, Mohammad Ali Amani, Hesam Kamyab, Shreeshivadasan Chelliapan. Graphene oxide-enhanced multiscale modeling of PGDLLA/P(lLA-co-ɛ-CL)/PCL interfacial debonding: investigating rheological and mechanical properties, compatibility, and morphology. 2025; 35(2), 553-573. Available from: doi:10.1007/s42823-024-00793-3

Ehsan Vafa, Mohammad Barghamadi, Somayeh Parham, Katayoon Rezaeeparto, Mohammad Bagher Zarei, Mohammad Javad Azizli, Mohammad Ali Amani, Hesam Kamyab and Shreeshivadasan Chelliapan. "Graphene oxide-enhanced multiscale modeling of PGDLLA/P(lLA-co-ɛ-CL)/PCL interfacial debonding: investigating rheological and mechanical properties, compatibility, and morphology" Carbon Letters 35, no.2 (2025) : 553-573.doi: 10.1007/s42823-024-00793-3