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@article{ART003274517},
author={Xinyu Xiao and Mingyue Li and Guangmeng Chen and Weihua Zhou and Weiwei Zhao and Xiaoqing Liu},
title={Self-supporting laser-induced graphene-based electrodes for efficient OER and 5-hydroxymethylfurfural oxidation},
journal={Carbon Letters},
issn={1976-4251},
year={2025},
volume={35},
number={6},
pages={2703-2716},
doi={10.1007/s42823-025-00948-w}

TY - JOUR
AU - Xinyu Xiao
AU - Mingyue Li
AU - Guangmeng Chen
AU - Weihua Zhou
AU - Weiwei Zhao
AU - Xiaoqing Liu
TI - Self-supporting laser-induced graphene-based electrodes for efficient OER and 5-hydroxymethylfurfural oxidation
JO - Carbon Letters
PY - 2025
VL - 35
IS - 6
PB - Korean Carbon Society
SP - 2703
EP - 2716
SN - 1976-4251
AB - Improving the oxygen evolution reaction (OER) performance or replacing OER with the value-added conversion of biomass is of great significance for the green hydrogen energy production. In this work, bimetallic species-decorated laser-induced graphene (LIG) was fabricated and demonstrated as the self-supported electrodes towards efficient OER and 5-hydroxymethylfurfural oxidation reaction (HMFOR). Three-dimensional LIG was obtained via one-step irradiation process under ambient conditions, and active metal species were then introduced through electrodeposition, with Ni-based catalyst as the primary catalytic material and Fe and Co as modified metals. Among, LIG-NiFe electrode achieved an extremely low overpotential of 241.7 mV at a current density of 20 mA/cm2 for OER and demonstrated long-term stability. This could be attributed to the promoted formation of Ni3+ active centers by Fe modified and the intrinsic porous structure of LIG providing an enhanced surface area. As for LIG-NiCo, due to the low onset potential of Co for HMF, it could achieve 99.6% HMF conversion and yielded value-added 2, 5-furandicarboxylic acid (FDCA) with a selectivity of 87.1%. Coupled with the merit of facile fabrication of LIG framework, this study demonstrates that LIG-based electrodes assume great practical application value in electrocatalytic reactions.
KW - Laser-induced graphene;Self-supporting;Oxygen evolution reaction;5-Hydroxymethylfurfural oxidation reaction
DO - 10.1007/s42823-025-00948-w
ER -

Xinyu Xiao, Mingyue Li, Guangmeng Chen, Weihua Zhou, Weiwei Zhao and Xiaoqing Liu. (2025). Self-supporting laser-induced graphene-based electrodes for efficient OER and 5-hydroxymethylfurfural oxidation. Carbon Letters, 35(6), 2703-2716.

Xinyu Xiao, Mingyue Li, Guangmeng Chen, Weihua Zhou, Weiwei Zhao and Xiaoqing Liu. 2025, "Self-supporting laser-induced graphene-based electrodes for efficient OER and 5-hydroxymethylfurfural oxidation", Carbon Letters, vol.35, no.6 pp.2703-2716. Available from: doi:10.1007/s42823-025-00948-w

Xinyu Xiao, Mingyue Li, Guangmeng Chen, Weihua Zhou, Weiwei Zhao, Xiaoqing Liu "Self-supporting laser-induced graphene-based electrodes for efficient OER and 5-hydroxymethylfurfural oxidation" Carbon Letters 35.6 pp.2703-2716 (2025) : 2703.

Xinyu Xiao, Mingyue Li, Guangmeng Chen, Weihua Zhou, Weiwei Zhao, Xiaoqing Liu. Self-supporting laser-induced graphene-based electrodes for efficient OER and 5-hydroxymethylfurfural oxidation. 2025; 35(6), 2703-2716. Available from: doi:10.1007/s42823-025-00948-w

Xinyu Xiao, Mingyue Li, Guangmeng Chen, Weihua Zhou, Weiwei Zhao and Xiaoqing Liu. "Self-supporting laser-induced graphene-based electrodes for efficient OER and 5-hydroxymethylfurfural oxidation" Carbon Letters 35, no.6 (2025) : 2703-2716.doi: 10.1007/s42823-025-00948-w

Xinyu Xiao; Mingyue Li; Guangmeng Chen; Weihua Zhou; Weiwei Zhao; Xiaoqing Liu. Self-supporting laser-induced graphene-based electrodes for efficient OER and 5-hydroxymethylfurfural oxidation. Carbon Letters, 35(6), 2703-2716. doi: 10.1007/s42823-025-00948-w

Xinyu Xiao; Mingyue Li; Guangmeng Chen; Weihua Zhou; Weiwei Zhao; Xiaoqing Liu. Self-supporting laser-induced graphene-based electrodes for efficient OER and 5-hydroxymethylfurfural oxidation. Carbon Letters. 2025; 35(6) 2703-2716. doi: 10.1007/s42823-025-00948-w

Xinyu Xiao, Mingyue Li, Guangmeng Chen, Weihua Zhou, Weiwei Zhao, Xiaoqing Liu. Self-supporting laser-induced graphene-based electrodes for efficient OER and 5-hydroxymethylfurfural oxidation. 2025; 35(6), 2703-2716. Available from: doi:10.1007/s42823-025-00948-w

Xinyu Xiao, Mingyue Li, Guangmeng Chen, Weihua Zhou, Weiwei Zhao and Xiaoqing Liu. "Self-supporting laser-induced graphene-based electrodes for efficient OER and 5-hydroxymethylfurfural oxidation" Carbon Letters 35, no.6 (2025) : 2703-2716.doi: 10.1007/s42823-025-00948-w